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Rosiello, Angelo
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Rosiello, Angelo
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- PublicationOpen AccessMeasuring and interpreting CO2 fluxes at regional scale: the case of the Apennines, Italy(Geological society of London, 2019)
; ; ; ; ; ; ;; ; ; ;Tectonically active regions are often characterized by large amounts of carbon dioxide degassing, and estimation of the total CO2 discharged to the atmosphere from tectonic structures, hydrothermal systems and inactive volcanic areas is crucial for the definition of present-day global Earth degassing. The carbon balance of regional aquifers is a powerful tool to quantify the diffuse degassing of deep inorganic carbon sources because the method integrates the CO2 flux over large areas. Its application to peninsular Italy shows that the region is characterized by specific CO2 fluxes higher than the baseline determined for the geothermal regions of the world, and that the amount of endogenous CO2 discharged through diffuse regional degassing (c. 2.1 × 1011 mol a−1) is the major component of the geological CO2 budget of Italy, definitely prevailing over the CO2 discharged by Italian active volcanoes and volcanoes with hydrothermal activity. Furthermore, the positive correlation between geothermal heat and deep CO2 dissolved in the groundwater of central Italy suggests that (1) the geothermal heat is transported into the aquifers by the same hot CO2-rich fluids causing the Italian CO2 anomaly and (2) the advective heat flow is the dominant form of heat transfer of the region.176 83 - PublicationOpen AccessCorrelation between tectonic CO2 Earth degassing and seismicity is revealed by a 10-year record in the Apennines, Italy(2020-08)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; Deep CO2 emissions characterize many nonvolcanic, seismically active regions worldwide, and the involvement of deep CO2 in the earthquake cycle is now generally recognized. However, no long-time records of such emissions have been published, and the temporal relations between earthquake occurrence and tectonic CO2 release remain enigmatic. Here, we report a 10-year record (2009-2018) of tectonic CO2 flux in the Apennines (Italy) during intense seismicity. The gas emission correlates with the evolution of the seismic sequences: Peaks in the deep CO2 flux are observed in periods of high seismicity and decays as the energy and number of earthquakes decrease. We propose that the evolution of seismicity is modulated by the ascent of CO2 accumulated in crustal reservoirs and originating from the melting of subducted carbonates. This large-scale, continuous process of CO2 production favors the formation of overpressurized CO2-rich reservoirs potentially able to trigger earthquakes at crustal depth.490 111 - PublicationOpen AccessActive degassing of crustal CO2 in areas of tectonic collision: A case study from the Pollino and Calabria sectors (Southern Italy)(2022)
; ; ; ; ; ; ; ; ; ;; ;; ; ;; ;Carbon dioxide (CO2) is released from the Earth’s interior into the atmosphere through both volcanic and non-volcanic sources in a variety of tectonic settings. A quantitative understanding of CO2 outgassing fluxes in different geological settings is thus critical for decoding the link between the global carbon budget and different natural processes (e.g., volcanic eruption and earthquake nucleation) and the effects on the climate evolution over geological time. It has recently been proposed that CO2 degassing from non-volcanic areas is a major component of the natural CO2 emission budget, but available data are still sparse and incomplete. Here, we report the results of a geochemical survey aimed at quantifying CO2 emissions through cold and thermal springs of the tectonically active Pollino Massif and Calabrian arc (Southern Italy). The chemical ad isotopic (He and C) composition of fifty-five dissolved gas samples allows to identify two different domains: 1) a shallow system dominated by gas components of atmospheric signature (helium, hereafter He) and biogenic origin (C), and 2) a deeper system in which crustal/deep fluids (CO2 and He) are dominant. The measured He isotope ratios range from 0.03 to 1.1 Ra (where Ra is the He isotopic ratio in the atmosphere) revealing a variable atmospheric contamination. Furthermore, the He isotopic data indicate the presence of traces of mantle He contributions (2%–3%) in the thermal groundwater. The prevailing low R/Ra values reflect the addition of crustal radiogenic 4He during groundwater circulation. Using helium and carbon isotope data, we explore the possible sources of fluids and the secondary processes (dissolution/ precipitation) that act to modify the chemistry of pristine volatiles. For the thermal springs, we estimate a deep C output of 2.3 x 107 to 6.1 x 108 mol year−1. These values correspond to deep CO2 fluxes per square km comparable with those estimated in several active and inactive volcanic areas and in continental regions affected by metamorphic CO2 degassing (e.g., the southern margin of the Tibetan Plateau).252 27 - PublicationRestrictedTriponzo: a thermal system in a cold area of the Apennines (Italy)Bagni di Triponzo thermal springs, characterised by a Ca-SO4 composition and temperatures up to 30°C, are located in the eastern sector of Umbria region in the Umbria-Marche Apennine (central Italy). The region is characterised by a low geothermal gradient and low conductive heat flux and the composition of Triponzo thermal waters significantly differs with respect to the cold waters circulating in the surrounding areas. The origin of the heat transported by the waters of the Triponzo springs is mainly due to a deep component, characterised by high CO2 and He contents, coming from a deeper reservoir, rising along normal faults and mixing with infiltrating waters of meteoric origin. The total amount of thermal water discharged by the system is about 34 L s-1. According to the ternary SO4-2-F--HCO3- geoindicator for carbonate-evaporite reservoirs, the fluids at reservoir condition are charcterised by a partial pressure of CO2 about 0.5 bar and a temperature between 70-75°C whereas the Silica geothermometers give a temperature about 62°C. The computed thermal energy transported by advection and discharged at the surface by Triponzo springs is about 3.71×1011 ± 0.56×1011 J/day.
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