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The global methane budget 2000–2012

Author(s)
Saunois, Marielle  
Bousquet, Philippe  
Poulter, Ben  
Peregon, Anna  
Ciais, Philippe  
Canadell, Josep G.  
Dlugokencky, Edward J.  
Etiope, Giuseppe  
Istituto Nazionale di Geofisica e Vulcanologia (INGV), Sezione Roma2, Roma, Italia  
Bastviken, David  
Houweling, Sander  
Janssens-Maenhout, Greet  
Tubiello, Francesco N.  
Castaldi, Simona  
Jackson, Robert B.  
Alexe, Mihai  
Arora, Vivek K.  
Beerling, David J.  
Bergamaschi, Peter  
Blake, Donald R.  
Brailsford, Gordon  
Brovkin, Victor  
Bruhwiler, Lori  
Crevoisier, Cyril  
Crill, Patrick  
Covey, Kristofer  
Curry, Charles  
Frankenberg, Christian  
Gedney, Nicola  
Höglund-Isaksson, Lena  
Ishizawa, Misa  
Ito, Akihiko  
Joos, Fortunat  
Kim, Heon-Sook  
Kleinen, Thomas  
Krummel, Paul  
Lamarque, Jean-François  
Langenfelds, Ray  
Locatelli, Robin  
Machida, Toshinobu  
Maksyutov, Shamil  
McDonald, Kyle C.  
Marshall, Julia  
Melton, Joe R.  
Morino, Isamu  
Naik, Vaishali  
O'Doherty, Simon  
Parmentier, Frans-Jan W.  
Patra, Prabir K.  
Peng, Changhui  
Peng, Shushi  
Peters, Glen P.  
Pison, Isabelle  
Prigent, Catherine  
Prinn, Ronald  
Ramonet, Michel  
Riley, William J.  
Saito, Makoto  
Santini, Monia  
Schroeder, Ronny  
Simpson, Isobel J.  
Spahni, Renato  
Steele, Paul  
Takizawa, Atsushi  
Thornton, Brett F.  
Tian, Hanqin  
Tohjima, Yasunori  
Viovy, Nicolas  
Voulgarakis, Apostolos  
van Weele, Michiel  
van der Werf, Guido R.  
Weiss, Ray  
Wiedinmyer, Christine  
Wilton, David J.  
Wiltshire, Andy  
Worthy, Doug  
Wunch, Debra  
Xu, Xiyan  
Yoshida, Yukio  
Zhang, Bowen  
Zhang, Zhen  
Zhu, Qiuan  
Language
English
Obiettivo Specifico
6A. Geochimica per l'ambiente
Status
Published
JCR Journal
JCR Journal
Journal
Earth System Science Data  
Issue/vol(year)
/8 (2016)
Pages (printed)
697–751
Date Issued
2016
DOI
10.5194/essd-8-697-2016
URI
https://www.earth-prints.org/handle/2122/10744
Abstract
The global methane (CH4) budget is becoming an increasingly important component for managing
realistic pathways to mitigate climate change. This relevance, due to a shorter atmospheric lifetime and a stronger warming potential than carbon dioxide, is challenged by the still unexplained changes of atmospheric CH4 over the past decade. Emissions and concentrations of CH4 are continuing to increase, making CH4 the second most important human-induced greenhouse gas after carbon dioxide. Two major difficulties in reducing uncertainties come from the large variety of diffusive CH4 sources that overlap geographically, and from the destruction of CH4 by the very short-lived hydroxyl radical (OH). To address these difficulties, we have established a consortium of multi-disciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate research on the methane cycle, and producing regular ( biennial) updates of the global methane budget. This consortium includes atmospheric physicists and chemists, biogeochemists of surface and marine emissions, and socio-economists who study anthropogenic emissions. Following Kirschke et al. (2013), we propose here the first version of a living review paper that integrates results of top-down studies (exploiting atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up models, inventories and data-driven approaches (including process-based models for estimating land surface emissions and atmospheric chemistry, and inventories for anthropogenic emissions, data-driven extrapolations). For the 2003–2012 decade, global methane emissions are estimated by top-down inversions at 558 TgCH4 yr􀀀1, range 540–568. About 60% of global emissions are anthropogenic (range 50–65 %). Since 2010, the bottom-up global emission inventories have been closer to methane emissions in the most carbon intensive Representative Concentrations Pathway (RCP8.5) and higher than all other RCP scenarios. Bottom-up
approaches suggest larger global emissions (736 TgCH4 yr􀀀1, range 596–884) mostly because of larger natural emissions from individual sources such as inland waters, natural wetlands and geological sources. Considering the atmospheric constraints on the top-down budget, it is likely that some of the individual emissions reported by the bottom-up approaches are overestimated, leading to too large global emissions. Latitudinal data from top-down emissions indicate a predominance of tropical emissions ( 64% of the global budget, < 30 N) as compared to mid ( 32 %, 30–60 N) and high northern latitudes ( 4 %, 60–90 N). Top-down inversions consistently infer lower emissions in China ( 58 TgCH4 yr􀀀1, range 51–72, 􀀀14 %) and higher emissions in Africa (86 TgCH4 yr􀀀1, range 73–108, C19 %) than bottom-up values used as prior estimates. Overall, uncertainties for anthropogenic emissions appear smaller than those from natural sources, and the uncertainties on source categories appear larger for top-down inversions than for bottom-up inventories and models.
The most important source of uncertainty on the methane budget is attributable to emissions from wetland and other inland waters. We show that the wetland extent could contribute 30–40% on the estimated range for wetland emissions. Other priorities for improving the methane budget include the following: (i) the development of process-based models for inland-water emissions, (ii) the intensification of methane observations at local scale (flux measurements) to constrain bottom-up land surface models, and at regional scale (surface networks and satellites) to constrain top-down inversions, (iii) improvements in the estimation of atmospheric loss by OH, and (iv) improvements of the transport models integrated in top-down inversions. The data presented here can be downloaded from the Carbon Dioxide Information Analysis Center (http://doi.org/10.3334/CDIAC/GLOBAL_METHANE_BUDGET_2016_V1.1) and the Global Carbon Project.
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