Using a scale model room to assess the contribution of building material of volcanic origin to indoor radon
Author(s)
Language
English
Obiettivo Specifico
6A. Geochimica per l'ambiente e geologia medica
Status
Published
JCR Journal
JCR Journal
Peer review journal
Yes
Journal
Issue/vol(year)
2/65 (2020)
Pages (printed)
71-76
Date Issued
2020
Subjects
Using a scale model room to assess the contribution of building material of volcanic origin to indoor radon
Abstract
In the frame of Radon rEal time monitoring System and Proactive Indoor Remediation (RESPIRE),
a LIFE 2016 project funded by the European Commission, the contribution of building materials of volcanic
origin to indoor radon concentration was investigated. First, total gamma radiation and related outdoor dose
rates of geological materials in the Caprarola area (Central Italy) were measured to defi ne main sources of radiation. Second, Rn-222 and Rn-220 exhalation rates of these rocks used as building materials were measured using an accumulation chamber connected in a closed loop with a RAD7 radon monitor. Among others, the very porous “Tufo di Gallese” ignimbrite provided the highest values. This material was then used to construct a scale model room of 62 cm × 50 cm × 35 cm (inner length × width × height, respectively) to assess experimental radon and thoron activity concentration at equilibrium and study the effects of climatic conditions and different
coatings on radon levels. A fi rst test was carried out at ambient temperature to determine experimental Rn-222 and Rn-220 equilibrium activities in the model room, not covered with plaster or other coating materials. Experimental Rn-222 equilibrium was recorded in just two days demonstrating that the room “breaths”, exchanging air with the outdoor environment. This determines a dilution of indoor radon concentration. Other experiments showed that inner covers (such as plasterboard and different kinds of paints) partially infl uence Rn-222 but entirely cut the short-lived Rn-220. Finally, decreases in ambient temperature reduce radon exhalation from building material and, in turn, indoor activity concentration.
a LIFE 2016 project funded by the European Commission, the contribution of building materials of volcanic
origin to indoor radon concentration was investigated. First, total gamma radiation and related outdoor dose
rates of geological materials in the Caprarola area (Central Italy) were measured to defi ne main sources of radiation. Second, Rn-222 and Rn-220 exhalation rates of these rocks used as building materials were measured using an accumulation chamber connected in a closed loop with a RAD7 radon monitor. Among others, the very porous “Tufo di Gallese” ignimbrite provided the highest values. This material was then used to construct a scale model room of 62 cm × 50 cm × 35 cm (inner length × width × height, respectively) to assess experimental radon and thoron activity concentration at equilibrium and study the effects of climatic conditions and different
coatings on radon levels. A fi rst test was carried out at ambient temperature to determine experimental Rn-222 and Rn-220 equilibrium activities in the model room, not covered with plaster or other coating materials. Experimental Rn-222 equilibrium was recorded in just two days demonstrating that the room “breaths”, exchanging air with the outdoor environment. This determines a dilution of indoor radon concentration. Other experiments showed that inner covers (such as plasterboard and different kinds of paints) partially infl uence Rn-222 but entirely cut the short-lived Rn-220. Finally, decreases in ambient temperature reduce radon exhalation from building material and, in turn, indoor activity concentration.
Sponsors
This research was accomplished in the frame of RESPIRE, a LIFE 2016 project funded by the European Commission. GRANT AGREEMENT N. LIFE 16ENV/IT/000553
References
1. National Council on Radiation Protection and Measurements. (2009). Ionizing radiation exposure of the population of the United States. Bethesda, MD: NCRP. (Report no. 160).
2. Bruno, R. C. (1983). Sources of indoor radon in houses: A review. Journal of the Air Pollution Control Association, 33(2), 105–109. DOI: 10.1080/00022470.1983.10465550.
3. Ruggiero, L., Bigi, S., Ciotoli, G., Galli, G., Giustini, F., Lombardi, S., Lucchetti, C., Pizzino, L., Sciarra, A.,
Sirianni, P., Tartarello, M. C., & Voltaggio, M. (2018). Relationships between geogenic radon potential and
gamma ray maps with indoor radon levels at Caprarola municipality (central Italy). In GARMM – 14. International Workshop on the Geological Aspects of Radon Risk Mapping, 18–20 September 2018, Prague,
Czech Republic. (extended abstract).
4. Tuccimei, P., Castelluccio, M., Soligo, M., & Moroni, M. (2009). Radon exhalation rates of building materials: experimental, analytical protocol and classifi cation criteria. In D. N. Cornejo & J. L. Haro (Eds.), Building materials: Properties, performance and applications (pp. 259–273). Hauppauge, NY: Nova Science Publishers.
5. Lucchetti, C., Briganti, A., Castelluccio, M., Galli, G., Santilli, S., Soligo, M., & Tuccimei, P. (2019). Integrating radon and thoron fl ux data with gamma radiation mapping in radon-prone areas. The case of
volcanic outcrops in a highly-urbanized city (Roma, Italy). J. Environ. Radioact., 202, 41–50. DOI: 10.1016/j.jenvrad.2019.02.004.
6. Tuccimei, P., Moroni, M., & Norcia, D. (2006). Simultaneous determination of 222Rn and 220Rn exhalation
rates from building materials used in Central Italy with accumulation chambers and a continuous solid state alpha detector: infl uence of particle size, humidity and precursors concentration. Appl. Radiat. Isot., 64(2), 254–263.
7. Wiegand, J. (2001). A guideline for the evaluation of the soil radon potential based on geogenic and anthropogenic parameters. Environ. Geol., 40, 949–963.
8. Scarciglia, F., Tuccimei, P., Vacca, A., Barca, D., Pulice, I., Salzano, R., & Soligo, M. (2011). Soil genesis, morphodynamic processes and chronological implications in two soil transects of SE Sardinia, Italy: traditional pedological study coupled with laser ablation ICP-MS and radionuclide analyses. Geoderma, 162, 39–64. DOI: 10.1016/j.geoderma.2011.01.004.
9. De Simone, G., Lucchetti, C., Galli, G., & Tuccimei, P. (2016). Correcting for H2O interference using
electrostatic collection-based silicon detectors. J. Environ. Radioact., 162/163, 146–153. DOI: 10.1016/j.
jenvrad.2016.05.021.
10. Tuccimei, P., Castelluccio, M., Moretti, S., Mollo, S., Vinciguerra, S., & Scarlato, P. (2011). Thermal
enhancement of radon emission from rocks. Implications for laboratory experiments under increasing
deformation. In B. Veress & J. Szigethy (Eds.), Horizons in earth science research (Vol. 4, Chapter 9, pp. 247–256). Hauppauge, NY: Nova Science Publishers
2. Bruno, R. C. (1983). Sources of indoor radon in houses: A review. Journal of the Air Pollution Control Association, 33(2), 105–109. DOI: 10.1080/00022470.1983.10465550.
3. Ruggiero, L., Bigi, S., Ciotoli, G., Galli, G., Giustini, F., Lombardi, S., Lucchetti, C., Pizzino, L., Sciarra, A.,
Sirianni, P., Tartarello, M. C., & Voltaggio, M. (2018). Relationships between geogenic radon potential and
gamma ray maps with indoor radon levels at Caprarola municipality (central Italy). In GARMM – 14. International Workshop on the Geological Aspects of Radon Risk Mapping, 18–20 September 2018, Prague,
Czech Republic. (extended abstract).
4. Tuccimei, P., Castelluccio, M., Soligo, M., & Moroni, M. (2009). Radon exhalation rates of building materials: experimental, analytical protocol and classifi cation criteria. In D. N. Cornejo & J. L. Haro (Eds.), Building materials: Properties, performance and applications (pp. 259–273). Hauppauge, NY: Nova Science Publishers.
5. Lucchetti, C., Briganti, A., Castelluccio, M., Galli, G., Santilli, S., Soligo, M., & Tuccimei, P. (2019). Integrating radon and thoron fl ux data with gamma radiation mapping in radon-prone areas. The case of
volcanic outcrops in a highly-urbanized city (Roma, Italy). J. Environ. Radioact., 202, 41–50. DOI: 10.1016/j.jenvrad.2019.02.004.
6. Tuccimei, P., Moroni, M., & Norcia, D. (2006). Simultaneous determination of 222Rn and 220Rn exhalation
rates from building materials used in Central Italy with accumulation chambers and a continuous solid state alpha detector: infl uence of particle size, humidity and precursors concentration. Appl. Radiat. Isot., 64(2), 254–263.
7. Wiegand, J. (2001). A guideline for the evaluation of the soil radon potential based on geogenic and anthropogenic parameters. Environ. Geol., 40, 949–963.
8. Scarciglia, F., Tuccimei, P., Vacca, A., Barca, D., Pulice, I., Salzano, R., & Soligo, M. (2011). Soil genesis, morphodynamic processes and chronological implications in two soil transects of SE Sardinia, Italy: traditional pedological study coupled with laser ablation ICP-MS and radionuclide analyses. Geoderma, 162, 39–64. DOI: 10.1016/j.geoderma.2011.01.004.
9. De Simone, G., Lucchetti, C., Galli, G., & Tuccimei, P. (2016). Correcting for H2O interference using
electrostatic collection-based silicon detectors. J. Environ. Radioact., 162/163, 146–153. DOI: 10.1016/j.
jenvrad.2016.05.021.
10. Tuccimei, P., Castelluccio, M., Moretti, S., Mollo, S., Vinciguerra, S., & Scarlato, P. (2011). Thermal
enhancement of radon emission from rocks. Implications for laboratory experiments under increasing
deformation. In B. Veress & J. Szigethy (Eds.), Horizons in earth science research (Vol. 4, Chapter 9, pp. 247–256). Hauppauge, NY: Nova Science Publishers
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