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Aiuppa, Alessandro
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Aiuppa, Alessandro
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- PublicationOpen AccessExcess degassing drives long-term volcanic unrest at Nevado del Ruiz(2024-01-12)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;; ; This study combines volcanic gas compositions, SO2 flux and satellite thermal data collected at Nevado del Ruiz between 2018 and 2021. We find the Nevado del Ruiz plume to have exhibited relatively steady, high CO2 compositions (avg. CO2/ST ratios of 5.4 ± 1.9) throughout. Our degassing models support that the CO2/ST ratio variability derives from volatile exsolution from andesitic magma stored in the 1-4 km depth range. Separate ascent of CO2-rich gas bubbles through shallow (< 1 km depth), viscous, conduit resident magma causes the observed excess degassing. We infer that degassing of ~ 974 mm3 of shallow (1-4 km) stored magma has sourced the elevated SO2 degassing recorded during 2018-2021 (average flux ~ 1548 t/d). Of this, only < 1 mm3 of magma have been erupted through dome extrusion, highlighting a large imbalance between erupted and degassed magma. Escalating deep CO2 gas flushing, combined with the disruption of passive degassing, through sudden accumulation and pressurization of bubbles due to lithostatic pressure, may accelerate volcanic unrest and eventually lead to a major eruption.44 24 - PublicationOpen AccessA SO2 flux study of the Etna volcano 2020–2021 paroxysmal sequences(2023-06-01)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; The persistent open-vent degassing of Mt. Etna is often punctuated by monthslong paroxysmal sequences characterized by episodes of violent Strombolian to lava fountaining activity. Understanding these gas-fueled transitions from quiescence to eruption requires routine measurement of gas fluxes. Here, we report SO2 flux measurements, obtained from a permanent UV camera system, collected over a two-year-long period spanning two paroxysmal sequences of Etna’s New South East Crater (NSEC) in December 2020/April 2021 and May/ October 2021. In both cases, SO2 flux increased from ≤ 3250 Mg/day during “ordinary” activity to ≥ 4200 Mg/day. We interpret these distinct SO2 degassing regimes in light of seismic and thermal observations and drawing on numerical simulations of sulfur degassing constrained by parental melt sulfur contents in Etna’s hawaiites. We find that initiation of a paroxysmal sequence results from an approximate doubling of the time-averaged rate of magma supply (and degassing) above the sulfur exsolution level (~150 MPa pressure), to >4m3/s. This corroborates recent models that argue for the triggering of paroxysmal sequences by escalating supply of volatile-rich magma to a reservoir ~3–4 km below the summit region. The non-stationary nature of magma flow and volcanic degassing we identify highlights the need for sustained surveillance to characterize long-term atmospheric budgets of volcanic volatiles151 25 - PublicationOpen AccessTemporal Variability in Gas Emissions at Bagana Volcano Revealed by Aerial, Ground, and Satellite Observations(2023)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;; Bagana is a remote, highly active volcano, located on Bougainville Island in southeastern Papua New Guinea. The volcano has exhibited sustained and prodigious sulfur dioxide gas emissions in recent decades, accompanied by frequent episodes of lava extrusion. The remote location of Bagana and its persistent activity have made it a valuable case study for satellite observations of active volcanism. This remoteness has also left many features of Bagana relatively unexplored. Here, we present the first measurements of volcanic gas composition, achieved by unoccupied aerial system (UAS) flights through the volcano's summit plume, and a payload comprising a miniaturized MultiGAS. We combine our measurements of the molar CO2/SO2 ratio in the plume with coincident remote sensing measurements (ground- and satellite-based) of SO2 emission rate to compute the first estimate of CO2 flux at Bagana. We report low SO2 and CO2 fluxes at Bagana from our fieldwork in September 2019, ∼320 ± 76 td −1 and ∼320 ± 84 td −1, respectively, which we attribute to the volcano's low level of activity at the time of our visit. We use satellite observations to demonstrate that Bagana's activity and emissions behavior are highly variable and advance the argument that such variability is likely an inherent feature of many volcanoes worldwide and yet is inadequately captured by our extant volcanic gas inventories, which are often biased to sporadic measurements. We argue that there is great value in the use of UAS combined with MultiGAS-type instruments for remote monitoring of gas emissions from other inaccessible volcanoes.48 28 - PublicationOpen AccessExceptional eruptive CO2 emissions from intra-plate alkaline magmatism in the Canary volcanic archipelago(2023)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;Alkaline mafic magmas forming intra-plate oceanic islands are believed to be strongly enriched in CO2 due to low-degree partial melting of enriched mantle sources. However, until now, such CO2 enhancement has not been verified by measuring CO2 degassing during a subaerial eruption. Here, we provide evidence of highly CO2-rich gas emissions during the 86-day 2021 Tajogaite eruption of Cumbre Vieja volcano on La Palma Island, in the Canary archipelago. Our results reveal sustained high plume CO2/SO2 ratios, which, when combined with SO2 fluxes, melt inclusion volatile contents and magma production rates at explosive and effusive vents, imply a magmatic CO2 content of 4.5 ± 1.5 wt%. The amount of CO2 released during the 2021 eruptive activity was 28 ± 14 Mt CO2. Extrapolating to the volume of alkaline mafic magmas forming La Palma alone (estimated as 4000 km3 erupted over 11 Ma), we infer a maximum CO2 emission into the ocean and atmosphere of 1016 moles of CO2, equivalent to 20% of the eruptive CO2 emissions from a large igneous province eruption, suggesting that the formation of the Canary volcanic archipelago produced a CO2 emission of similar magnitude as a large igneous province.8 7 - PublicationOpen AccessRapid shifting of a deep magmatic source at Fagradalsfjall volcano, Iceland(2022-09)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;; Recent Icelandic rifting events have illuminated the roles of centralized crustal magma reservoirs and lateral magma transport1-4, important characteristics of mid-ocean ridge magmatism1,5. A consequence of such shallow crustal processing of magmas4,5 is the overprinting of signatures that trace the origin, evolution and transport of melts in the uppermost mantle and lowermost crust6,7. Here we present unique insights into processes occurring in this zone from integrated petrologic and geochemical studies of the 2021 Fagradalsfjall eruption on the Reykjanes Peninsula in Iceland. Geochemical analyses of basalts erupted during the first 50 days of the eruption, combined with associated gas emissions, reveal direct sourcing from a near-Moho magma storage zone. Geochemical proxies, which signify different mantle compositions and melting conditions, changed at a rate unparalleled for individual basaltic eruptions globally. Initially, the erupted lava was dominated by melts sourced from the shallowest mantle but over the following three weeks became increasingly dominated by magmas generated at a greater depth. This exceptionally rapid trend in erupted compositions provides an unprecedented temporal record of magma mixing that filters the mantle signal, consistent with processing in near-Moho melt lenses containing 107-108 m3 of basaltic magma. Exposing previously inaccessible parts of this key magma processing zone to near-real-time investigations provides new insights into the timescales and operational mode of basaltic magma systems.55 10 - PublicationOpen AccessShallow magma dynamics at open-vent volcanoes tracked by coupled thermal and SO2 observations(2022)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ;; ; ; ; ; ; ; ; ; ; ; ;Open-vent volcanic activity is typically sustained by ascent and degassing of shallow magma, in which the rate of magma supply to the upper feeding system largely exceeds the rate of magma eruption. Such unbalance between supplied (input) and erupted (output) magma rates is thought to result from steady, degassing-driven, convective magma overturning in a shallow conduit/feeding dyke. Here, we characterize shallow magma circulation at Stromboli volcano by combining independent observations of heat (Volcanic Radiative Power; via satellite images) and gas (SO2 , via UV camera) output in a temporal interval (from August 1, 2018 to April 30, 2020) encompassing the summer 2019 effusive eruption and two paroxysmal explosions (on July 3 and August 28, 2019). We show that, during the phase of ordinary strombolian explosive activity that preceded the 2019 effusive eruption, the average magma input rate (0.1-0.2 m3 /s) exceeds the magma eruption rate (0.001-0.01 m3 /s) by ∼2 orders of magnitude. Conversely, magma input and output rates converge to an average of ∼0.4 m3 /s during the summer 2019 summit effusion, implying an overall suppression of magma recycling back into the feeding system, and hence of excess degassing. We find that, during the effusive eruption, the peak in SO2 emissions lags behind the thermal emission peak by ∼27 days, suggesting that magma output, feeding the lava flow field, initially dominates over magma input in the conduit. We propose that this conduit mass unloading, produced by this initial phase of the effusive eruption, leads to an overall decompression (of up to 30 Pa/s) of the shallow plumbing system, ultimately causing ascent of less-dense, volatile-rich magma batch(es) from depth, enhanced explosive activity, and elevated SO2 fluxes culminating into a paroxysmal explosion on August 28. Our results demonstrate that combined analysis of thermal and SO2 flux time-series paves the way to improved understanding of shallow magmatic system dynamics at open-vent volcanoes, and of the transition from explosive to effusive activity regimes.35 42 - PublicationOpen AccessSpatio-temporal changes in degassing behavior at Stromboli volcano derived from two co-exposed SO2 camera stations(2022)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;; Improving volcanic gas monitoring techniques is central to better understanding open-vent, persistently degassing volcanoes. SO2 cameras are increasingly used in volcanic gas studies, but observations are commonly limited to one single camera alone viewing the volcanic plume from a specific viewing direction. Here, we report on high frequency (0.5 Hz) systematic measurements of the SO2 flux at Stromboli, covering a 1-year long observation period (June 2017-June 2018), obtained from two permanent SO2 cameras using the same automated algorithm, but imaging the plume from two different viewing directions. Our aim is to experimentally validate the robustness of automatic SO2 camera for volcano monitoring and to demonstrate the advantage of using two co-exposed SO2 camera stations to better capturing degassing dynamics at open-vent volcanoes. The SO2 flux time-series derived from the two SO2 camera stations exhibit good match, demonstrating the robustness of the automatic SO2 camera method. Our high-temporal resolution SO2 records resolve individual Strombolian explosions as transient, repetitive gas bursts produced by the sudden release of over pressurized gas pockets and scoriae. Calculations show that explosive degassing activity accounts for ∼10% of the total SO2 emission budget (dominated by passive degassing) during mild regular open-vent activity. We show that the temporal variations of the explosive SO2 flux go in tandem with changes in total SO2 flux and VLP seismicity, implicating some commonality in the source processes controlling passive degassing and explosive activity. We exploited the spatial resolution of SO2 camera to discriminate degassing at two distinct regions of the crater area, and to minimize biases due by the station position respect to the target plume. We find that the SO2 fluxes from southwest-central (SWCC) and northeast (NEC) crater areas oscillate coherently but those from the NEC are more sensitive to the changes in the volcanic intensity. We interpret this as due to preferential gas/magma channeling into the structurally weaker north-eastern portion of the crater terrace in response to increasing supply rate of buoyant, bubble-rich magma in the shallow plumbing system.97 29 - PublicationOpen AccessMafic magma feeds degassing unrest at Vulcano Island, Italy(2022)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ;; ; ; ;; ; ; ; ; ; ;The benign fuming activity of dormant volcanoes is punctuated by phases of escalating degassing activity that, on some occasions, ultimately prelude to eruption. However, understanding the drivers of such unrest is complicated by complex interplay between magmatic and hydrothermal processes. Some of the most comprehensively characterised degassing unrest have recently been observed at La Fossa cone on Vulcano Island, but whether or not these episodes involve new, volatile-rich ascending magma remains debated. Here, we use volcanic gas measurements, in combination with melt inclusion information, to propose that heightened sulphur dioxide flux during the intense fall 2021 La Fossa unrest is sourced by degassing of volatile-rich mafic magma. Calculations using a numerical model indicate observations are consistent with the unrest being triggered by the emplacement of ∼3·106 m3 of mafic magma at ∼4–5 km depth. Degassing of mafic magma is argued as a recurrent driver of unrest at dormant volcanoes worldwide.132 21 - PublicationOpen AccessVolcanic CO2 tracks the incubation period of basaltic paroxysms(2021-09-17)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; ; The ordinarily benign activity of basaltic volcanoes is periodically interrupted by violent paroxysmal explosions ranging in size from Hawaiian to Plinian in the most extreme examples. These paroxysms often occur suddenly and with limited or no precursors, leaving their causal mechanisms still incompletely understood. Two such events took place in summer 2019 at Stromboli, a volcano otherwise known for its persistent mild open-vent activity, resulting in one fatality and damage to infrastructure. Here, we use a post hoc analysis and reinterpretation of volcanic gas compositions and fluxes acquired at Stromboli to show that the two paroxysms were preceded by detectable escalations in volcanic plume CO2 degassing weeks to months beforehand. Our results demonstrate that volcanic gas CO2 is a key driver of explosions and that the preparatory periods ahead of explosions in basaltic systems can be captured by precursory CO2 leakage from deeply stored mafic magma.105 23 - PublicationOpen AccessLong-term gas observations track the early unrest phases of open-vent basaltic volcanoes(2021-04-26)
; ; ; ; ; ; ; ; ; ; ; ; ; ; ;; ; ; ;; ; At open-vent basaltic volcanoes, resolving the activity escalation that heralds larger, potentially harmful eruptions is challenged by the persistent mild ordinary activity, which often masks the precursory unrest signals related to heightened magma transport from depth. Gas (SO2 and CO2) fluxes at surface are controlled by rate of magma transport and degassing within the magma plumbing system, and thus constitute key parameters to infer deep magma budget and dynamics. Here, we use several year-long (2014-present) gas observations at Etna and Stromboli volcanoes, in Sicily, to provide new evidence for the utility of long-term instrumental gas monitoring in real-time detecting the early phase of unrest prior eruption, and for characterizing syn-eruptive dynamics. To this aim, we use information from a gas monitoring network of permanent ultraviolet (UV) cameras and automatic Multi-Gas instruments that, combined with geophysical observations, allow characterizing changes in degassing and eruptive dynamics at high temporal/spatial resolution. Our results show that the paroxysmal (lava fountaining) explosions that periodically interrupted persistent open-vent activity on Etna (during 2014-2020) were accompanied by systematic, repetitive SO2 emission patterns prior, during, and after eruptions. These allow us identifying the characteristic pre- syn- and post- eruptive degassing regimes, and to establish thresholds in the SO2 flux record that mark phases of unrest. On Stromboli, the much improved temporal/spatial resolution of UV cameras allows resolving the escalation of regular strombolian activity, and its concentration toward its North-east crater, that heralds onset of effusive eruptions. During effusive eruption, although magma level drops in the conduit and explosive summit activity ceases, UV camera observations can still detect explosive gas bursts deep in the conduit while no infrasonic activity is detected. Combining the UV camera-derived SO2 fluxes with CO2/SO2 ratio records measured by the Multi-Gas, the CO2 flux can be inferred. We find that such CO2 flux time-series can allow tracking degassing of deeply stored mafic magma months before Stromboli"s eruptions. We finally show that remotely sensed gas emission and thermal activity can be combined together to characterize the dynamics of shallow magmatic system prior to and during unrest, ultimately helping to define timing of magma re-charging events driving the eruptions.43 8