Bossew, Peter

Radon is a radioactive gas and a major source of ionizing radiation exposure for humans. Consequently, it can pose serious health threats when it accumulates in confined environments. In Europe, recent legislation has been adopted to address radon exposure in dwellings; this law establishes national reference levels and guidelines for defining Radon Priority Areas (RPAs). This study focuses on mapping the Geogenic Radon Potential (GRP) as a foundation for identifying RPAs and, consequently, assessing radon risk in indoor environments. Here, GRP is proposed as a hazard indicator, indicating the potential for radon to enter buildings from geological sources. Various approaches, including multivariate geospatial analysis and the application of artificial intelligence algorithms, have been utilised to generate continuous spatial maps of GRP based on point measurements. In this study, we employed a robust multivariate machine learning algorithm (Random Forest) to create the GRP map of the central sector of the Pusteria Valley, incorporating other variables from census tracts such as land use as a vulnerability factor, and population as an exposure factor to create the risk map. The Pusteria Valley in northern Italy was chosen as the pilot site due to its well-known geological, structural, and geochemical features. The results indicate that high Rn risk areas are associated with high GRP values, as well as residential areas and high population density. Starting with the GRP map (e.g., Rn hazard), a new geological-based definition of the RPAs is proposed as fundamental tool for mapping Collective Radon Risk Areas in line with the main objective of European regulations, which is to differentiate them from Individual Risk Areas.

This work highlights the importance of the Geogenic Radon Potential (GRP) component originated by degassing processes in fault zones. This Tectonically Enhanced Radon (TER) can increase radon concentration in soil gas and the inflow of radon in the buildings (Indoor Radon Concentrations, IRC). Although tectonically related radon enhancement is known in areas characterised by active faults, few studies have investigated radon migration processes in non-active fault zones. The Pusteria Valley (Bolzano, north-eastern Italy) represents an ideal geological setting to study the role of a non-seismic fault system in enhancing the geogenic radon. Here, most of the municipalities are characterised by high IRC. We performed soil gas surveys in three of these municipalities located along a wide section of the non-seismic Pusteria fault system characterised by a dense network of faults and fractures. Results highlight the presence of high Rn concentrations (up to 800 kBq·m-3) with anisotropic spatial patterns oriented along the main strike of the fault system. We calculated a Radon Activity Index (RAI) along north-south profiles across the Pusteria fault system and found that TER is linked to high fault geochemical activities. This evidence confirms that TER constitutes a significant component of GRP also along non-seismic faults.

Radon isotopes (222Rn, 220Rn) are noble, naturally occurring radioactive gases. They originate from the alpha decay of radium isotopes (226Ra, 224Ra), which occur in most materials in the environment, i.e. soil, rocks, raw and building materials. Radon is also found in ground and tap water. The two radon isotopes are chemically identical, but they have very different halflives: 3.82 days for radon (222Rn) and 56 seconds for thoron (220Rn). Thus, they behave very differently in the environment. Both isotopes are alpha-emitters; their decay products are polonium, bismuth and lead isotopes. The main source of radon in air (indoor or outdoor) is soil, where radon concentrations are very high and reach tens of Bq/m3. Radon release from soil into the atmosphere depends on radium (226Ra) concentration in soil, soil parameters (porosity, density, humidity) and weather conditions (e.g. air temperature and pressure, wind, precipitation). Outdoor radon concentrations are relatively low and change daily and seasonally. These changes may be used to study the movement of air masses and other climatic conditions. Radon gas enters buildings (homes, workplaces) through cracks, crevices and leaks that occur in foundations and connections between different materials in the building. This is due to temperature and pressure differences between indoors and outdoors. Indoor radon is the most important source of radiation exposure to the public, especially on ground floor. Radon and its decay products represent the main contributor to the effective dose of ionising radiation that people receive. Radon is generally considered as the second cause of increased risk of lung cancer (after smoking). The only way to assess indoor radon concentration is to make measurements. Different methods exist, but the most common one is to use track-etched detectors. Such detectors may be used to perform longterm (e.g. annual) measurements in buildings. The exposure time is important because indoor radon levels change daily and seasonally. Moreover, radon concentration shows a high spatial variation on a local scale, and is strongly connected with geological structure, building characteristics and ventilation habits of occupants. A European map of indoor radon concentration has been prepared and is displayed. It is derived from survey data received from 35 countries participating on a voluntary basis.